396 MHz CPA femtosecond laser system based on a single crystal fiber rod-type amplifier.

The paper presents the results of multiplying the repetition frequency of the seed source to 396 MHz using an extra-cavity fiber multiplication method. The single crystal fiber rod-type amplifier was able to boost the average output power to approximately 15.9 W. Using a transmission gratings-based pulse compressor, an average output power of 9.56 W was achieved, corresponding to a burst energy of up to 382 µJ and a compression efficiency of 81.7%. The shortest pulse duration was optimized to be 594 fs; however, an obvious pedestal was also observed. This system reduces the impact of nonlinear effects on the device by increasing the repetition frequency, thereby increasing the injection energy of a single process in industrial processing.

High quality stealth dicing of sapphire with a picosecond Bessel beam by controlling the polarization direction.

Sapphire is an important substrate material in optoelectronic devices, and it is also widely used as a touch screen panel. In order to achieve high quality cutting of sapphire, the stealth dicing of 500 µm thick sapphire by a picosecond Bessel beam is studied in this paper. The influences of laser polarization direction and process parameters on cutting section roughness were studied. By controlling the laser polarization direction, different crack propagation morphologies were obtained. When the polarization direction was vertical to the cutting path, the crack propagation path was straighter, and the sapphire had better cutting quality. The laser processing parameters, including burst mode, hole spacing, and pulse energy, had a significant impact on the cutting section roughness. When the polarization direction was vertical to the cutting path under the optimal process parameters, the cutting section was uniform and flat, with no recondensable particles, no ripples, and no chamfer, and an 89.7 nm average roughness of the cutting section could be obtained.

Observation of bound solitons generated by a figure-9 fiber laser in the 1 µm band.

The paper describes the observation of diverse bound-state patterns, including tightly bound states, loosely bound states, and composite bound states, in a figure-9 fiber laser. By performing dispersion management and using polarization-maintaining fibers with high gain coefficient, stable dispersion-managed solitons and bound solitons can be simultaneously generated. This work advances our understanding of complex soliton dynamics and presents a novel, to the best of our knowledge, approach for future applications of bound states. Additionally, the research involves integrated packaging, effectively enhancing overall work stability.

A Novel Surface Modification on Core-Shell Yellow Particles for Electrophoretic Display.

This paper reports the synthesis of yellow-charged particles with a core-shell structure by modifying yellow pigment 181 particles using an ionic liquid under the sol-gel and grafting methods. The core-shell particles were characterized using various methods, including energy-dispersive X-ray spectroscopy, Fourier-transform infrared spectroscopy, colorimetry, thermogravimetric analysis, and others. The changes in zeta potential and particle size before and after modification were also measured. The results demonstrate that the surface of the PY181 particles was successfully coated with SiO2 microspheres, resulting in weak color change but increased brightness. The shell layer also caused an increase in the particle size. Moreover, the modified yellow particles exhibited apparent electrophoretic response, indicating improved electrophoretic properties. The core-shell structure significantly enhanced the performance of organic yellow pigment PY181, making this method a practical modification approach. This method provides a novel way of improving the electrophoretic performance of color pigment particles that are challenging to directly connect with an ionic liquid, leading to the improved electrophoretic mobility of pigment particles. It is suitable for the surface modification of various pigment particles.

NaCl-Assisted Chemical Vapor Deposition of Large-Domain Bilayer MoS2 on Soda-Lime Glass.

In recent years, two-dimensional molybdenum disulfide (MoS2) has attracted extensive attention in the application field of next-generation electronics. Compared with single-layer MoS2, bilayer MoS2 has higher carrier mobility and has more promising applications for future novel electronic devices. Nevertheless, the large-scale low-cost synthesis of high-quality bilayer MoS2 still has much room for exploration, requiring further research. In this study, bilayer MoS2 crystals grown on soda-lime glass substrate by sodium chloride (NaCl)-assisted chemical vapor deposition (CVD) were reported, the growth mechanism of NaCl in CVD of bilayer MoS2 was analyzed, and the effects of molybdenum trioxide (Mo) mass and growth pressure on the growth of bilayer MoS2 under the assistance of NaCl were further explored. Through characterization with an optical microscope, atomic force microscopy and Raman analyzer, the domain size of bilayer MoS2 prepared by NaCl-assisted CVD was shown to reach 214 µm, which is a 4.2X improvement of the domain size of bilayer MoS2 prepared without NaCl-assisted CVD. Moreover, the bilayer structure accounted for about 85%, which is a 2.1X improvement of bilayer MoS2 prepared without NaCl-assisted CVD. This study provides a meaningful method for the growth of high-quality bilayer MoS2, and promotes the large-scale and low-cost applications of CVD MoS2.

Application of High Potential Electrophoretic Particles Modified with High Ionization Mono Ionic Liquid for Electrophoretic Displays.

The electrophoretic display (EPD) has attracted widespread attention due to its great visual perception, energy-saving, portability, and bistability. However, the EPD still has many problems in response time, colorization, etc., which limits its practical application. In this paper, novel blue electrophoretic particles were prepared with copper (II) phthalocyanine and high ionization 1-butyl-1-methyl piperidinium bromide mono ionic liquid. It was shown that electrophoretic particles dispersed in a non-polar tetrachloroethylene medium had high Zeta potential and electrophoretic mobility. At the same time, electrophoretic particles showed better dispersion stability. Finally, the prepared blue electrophoretic particles and white titanium dioxide particles were compounded to prepare blue and white dual-color electrophoretic dispersion. An EPD cell was made to test its performance. The results showed that the prepared blue and white dual-color electrophoretic dispersion could realize a reversible response. Piperidine mono ionic liquid increased the surface potential of copper (II) phthalocyanine from +30.50 mV to +60.27 mV, enhancing it by 97.61%. Therefore, we believed that modifying particles with high ionization mono ionic liquid had great applicability to the modification of electrophoretic particles, and blue particles prepared with piperidine mono ionic liquid as a charge control agent (CCA) were excellent candidates for EPDs.

A Novel Modification of Copper (II) Phthalocyanine Particles towards Electrophoretic Displays.

Electrophoretic display (EPD) is a popular display technology in recent years. The core of the EPD is electrophoretic particles, and its Zeta potential has an important impact on EPDs. In this work, a method using pyrrolidine mono ionic liquid was proposed to improve the Zeta potential of electrophoretic particles: Copper (II) phthalocyanine pigment was modified with mono ionic liquid 1-Butyl-1-methylpyrrolidinium bromide. The characterization results show that the mono ionic liquid had been successfully coated on pigment particles. At the same time, the dispersion and stability of particles were improved. The modified Copper (II) phthalocyanine pigment could be stably dispersed in tetrachloroethylene for more than 20 days. The Zeta potential increased from 32.42 mV to 49.91 mV, increasing by 53.95%. Finally, the prepared blue electrophoretic particles were compounded with white titanium dioxide to prepare blue and white dual-color electrophoretic dispersion, and then an EPD cell was designed to test its performance. The results show that the prepared electrophoretic dispersion can realize reversible reciprocating motion. Therefore, because of the unique structure and properties of pyrrolidine mono ionic liquids, the blue nanoparticles prepared with pyrrolidine ionic liquids as charge control agents in this study can be used as excellent candidate materials for EPD.

Effect of Back-Gate Voltage on the High-Frequency Performance of Dual-Gate MoS2 Transistors.

As an atomically thin semiconductor, 2D molybdenum disulfide (MoS2) has demonstrated great potential in realizing next-generation logic circuits, radio-frequency (RF) devices and flexible electronics. Although various methods have been performed to improve the high-frequency characteristics of MoS2 RF transistors, the impact of the back-gate bias on dual-gate MoS2 RF transistors is still unexplored. In this work, we study the effect of back-gate control on the static and RF performance metrics of MoS2 high-frequency transistors. By using high-quality chemical vapor deposited bilayer MoS2 as channel material, high-performance top-gate transistors with on/off ratio of 107 and on-current up to 179 µA/µm at room temperature were realized. With the back-gate modulation, the source and drain contact resistances decrease to 1.99 kΩ∙µm at Vbg = 3 V, and the corresponding on-current increases to 278 µA/µm. Furthermore, both cut-off frequency and maximum oscillation frequency improves as the back-gate voltage increases to 3 V. In addition, a maximum intrinsic fmax of 29.7 GHz was achieved, which is as high as 2.1 times the fmax without the back-gate bias. This work provides significant insights into the influence of back-gate voltage on MoS2 RF transistors and presents the potential of dual-gate MoS2 RF transistors for future high-frequency applications.

High-Performance CVD Bilayer MoS2 Radio Frequency Transistors and Gigahertz Mixers for Flexible Nanoelectronics.

Two-dimensional (2D) MoS2 have attracted tremendous attention due to their potential applications in future flexible high-frequency electronics. Bilayer MoS2 exhibits the advantages of carrier mobility when compared with monolayer mobility, thus making the former more suitable for use in future flexible high-frequency electronics. However, there are fewer systematical studies of chemical vapor deposition (CVD) bilayer MoS2 radiofrequency (RF) transistors on flexible polyimide substrates. In this work, CVD bilayer MoS2 RF transistors on flexible substrates with different gate lengths and gigahertz flexible frequency mixers were constructed and systematically studied. The extrinsic cutoff frequency (fT) and maximum oscillation frequency (fmax) increased with reducing gate lengths. From transistors with a gate length of 0.3 µm, we demonstrated an extrinsic fT of 4 GHz and fmax of 10 GHz. Furthermore, statistical analysis of 14 flexible MoS2 RF transistors is presented in this work. The study of a flexible mixer demonstrates the dependence of conversion gain versus gate voltage, LO power and input signal frequency. These results present the potential of CVD bilayer MoS2 for future flexible high-frequency electronics.

3D Hollow rGO Microsphere Decorated with ZnO Nanoparticles as Efficient Sulfur Host for High-Performance Li-S Battery.

Lithium-sulfur battery (LSB) will become the next generation energy storage device if its severe shuttle effect and sluggish redox kinetics can be effectively addressed. Here, a unique three-dimensional hollow reduced graphene oxide microsphere decorated with ZnO nanoparticles (3D-ZnO/rGO) is synthesized to decrease the dissolution of lithium polysulfide (LiPS) into the electrolyte. The chemical adsorption of ZnO on LiPS is combined with the physical adsorption of 3D-rGO microsphere to synergistically suppress the shuttle effect. The obtained 3D-ZnO/rGO can provide sufficient space for sulfur storage, and effectively alleviate the repeated volume changes of sulfur during the cycle. When the prepared S-3D-ZnO/rGO was used as the cathode in LSB, an initial discharge specific capacity of 1277 mAh g-1 was achieved at 0.1 C. After 100 cycles, 949 mAh g-1 can still be maintained. Even at 1 C, a reversible discharge specific capacity of 726 mAh g-1 was delivered.

Improve polarization topological order sorting with the diffractive splitting method.

Vector beams with different polarization topological orders (PTOs) are the eigenmodes of traditional optical fibers and are orthogonal to each other, so the PTO multiplexing channel is a promising candidate for the oncoming generation of optical communication. Here we demonstrate experimentally a PTO sorting system with high separation resolution based on the diffractive splitting (DS) method. Our experiments show that our design with the DS method helps to enhance the separation resolution to 77.5% from 58%, compared to a design without the application of a DS method. Theoretically, to increase the copy number can promote the separation resolution further. This Letter provides a high-resolution way to decode information from PTO division multiplexing.

Generation of terahertz vortex pulses without any need of manipulation in the terahertz region.

Converting a Gaussian mode to a vortex beam is much more inconvenient in the terahertz (THz) region than in the near-infrared (NIR) region due to underdevelopment of THz components and strong THz diffraction. This Letter reports the direct generation of THz vortex pulses by optical difference-frequency between two NIR chirped pulses with different topological charges (TCs). By designing a passive and transmissive device for a collinear NIR pulse pair with conjugated TCs, we have experimentally obtained stable THz vortex pulses with a TC value of 2 or -2. The process needs no THz components and so is flexible to be realized and has promising applications in the THz field.

Common-path spectral interferometry for single-shot terahertz electro-optics detection: publisher's note.

This publisher's note corrects an error in one of the authors' names and an error in one of the grant numbers in Opt. Lett.42, 4263 (2017).

Common-path spectral interferometry for single-shot terahertz electro-optics detection.

We propose a common-path spectral interferometer for single-shot terahertz (THz) electro-optics (EO) detection, where a probe pulse pair with orthogonal polarizations and a relative time delay are generated by simply using a birefringent plate. One of them, as the object, transmits through a THz EO crystal with THz phase modulation, while the other goes through the crystal without any phase imposed by target the THz field as the reference. The co-axial propagation of the pulse pair can effectively reduce the noises due to mechanical vibrations, air turbulences, and temperature fluctuations in the traditional non-common-path spectral interferometers. Our experiments show that, for a given target THz pulse field, the measured THz signals in a single-shot mode have a signal-to-noise ratio (SNR) of 41.2 with our THz common-path spectral interferometer, but 7.91 with a THz Mach-Zehnder spectral interferometer; thus, our design improves the SNR of the THz signal by about 5.2 times.

Two-step phase-shifting SPIDER.

Comprehensive characterization of ultrafast optical field is critical for ultrashort pulse generation and its application. This paper combines two-step phase-shifting (TSPS) into the spectral phase interferometry for direct electric-field reconstruction (SPIDER) to improve the reconstruction of ultrafast optical-fields. This novel SPIDER can remove experimentally the dc portion occurring in traditional SPIDER method by recording two spectral interferograms with π phase-shifting. As a result, the reconstructed results are much less disturbed by the time delay between the test pulse replicas and the temporal widths of the filter window, thus more reliable. What is more, this SPIDER can work efficiently even the time delay is so small or the measured bandwidth is so narrow that strong overlap happens between the dc and ac portions, which allows it to be able to characterize the test pulses with complicated temporal/spectral structures or narrow bandwidths.

Modified THz electro-optic sampling for high optical modulation depth, large dynamical range, and low background noises.

We present a modified THz electro-optic sampling method to combine the advantages of its two traditional counterparts at near 0° and 45° optical biases: excellent ability to cancel the background noises, high optical modulation, and large dynamical range. The first advantage results from the method's symmetrical layout to get dynamical noise cancellation. By setting the static birefringent phases of the two balanced beams with a pair of opposite numbers, our setup can record THz waveforms without distortion with its maximal modulation depth, thus optimal signal-to-noise ratio (SNR). The setting also releases the linearity of the measured signal from the static birefringence, thus enlarging greatly the linear dynamical range. For a given THz field, the recorded SNR with our setup, without a lock-in, is more than 10 times higher than that with the "crossed and balanced" design [IEEE Trans. Microwave Theory Tech. 47, 2644 (1999)].